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Exploring second coordination sphere effects in flavodiiron nitric oxide reductase model complexes

https://doi.org/10.1039/d3dt02828c

Bracken, Abigail J. ; Dong, Hai T. ; Lengel, Michael O. ; Lehnert, Nicolai ( November 2023 , Dalton Transactions)

In this paper, we explore the role of SCS H-bonding interactions in the activation of NO by diiron complexes. Diferrous dinitrosyl complexes were prepared and spectroscopically characterized, and their reactivity upon reduction was investigated.
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Free, publicly-accessible full text available November 28, 2024
Bacterial nitric oxide reductase (NorBC) models employing click chemistry

https://doi.org/10.1016/j.jinorgbio.2023.112280

Harland, Jill B. ; Samanta, Subhra ; Lehnert, Nicolai ( September 2023 , Journal of Inorganic Biochemistry)

Free, publicly-accessible full text available September 1, 2024
Preparation and Characterization of a Formally Ni IV –Oxo Complex with a Triplet Ground State and Application in Oxidation Reactions

https://doi.org/10.1021/jacs.2c10196

Karmalkar, Deepika G. ; Larson, Virginia A. ; Malik, Deesha D. ; Lee, Yong-Min ; Seo, Mi Sook ; Kim, Jin ; Vasiliauskas, Dovydas ; Shearer, Jason ; Lehnert, Nicolai ; Nam, Wonwoo ( December 2022 , Journal of the American Chemical Society)

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What Is the Right Level of Activation of a High-Spin {FeNO} 7 Complex to Enable Direct N–N Coupling? Mechanistic Insight into Flavodiiron NO Reductases

https://doi.org/10.1021/jacs.2c04292

Dong, Hai T. ; Camarena, Stephanie ; Sil, Debangsu ; Lengel, Michael O. ; Zhao, Jiyong ; Hu, Michael Y. ; Alp, E. Ercan ; Krebs, Carsten ; Lehnert, Nicolai ( September 2022 , Journal of the American Chemical Society)

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Synthesis and characterization of a model complex for flavodiiron NO reductases that stabilizes a diiron mononitrosyl complex

https://doi.org/10.1016/j.jinorgbio.2022.111723

Dong, Hai T. ; Zong, Yu ; Bracken, Abigail J. ; Lengel, Michael O. ; Kampf, Jeff W. ; Sil, Debangsu ; Krebs, Carsten ; Lehnert, Nicolai ( April 2022 , Journal of Inorganic Biochemistry)

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A Monohydrosulfidodinitrosyldiiron Complex That Generates N 2 O as a Model for Flavodiiron Nitric Oxide Reductases: Reaction Mechanism and Electronic Structure

https://doi.org/10.1021/acs.inorgchem.1c00429

Pal, Nabhendu ; White, Corey J. ; Demeshko, Serhiy ; Meyer, Franc ; Lehnert, Nicolai ; Majumdar, Amit ( November 2021 , Inorganic Chemistry)

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Distortion of the [FeNO] 2 Core in Flavodiiron Nitric Oxide Reductase Models Inhibits N–N Bond Formation and Promotes Formation of Unusual Dinitrosyl Iron Complexes: Implications for Catalysis and Reactivity

https://doi.org/10.1021/jacs.1c10388

White, Corey J. ; Lengel, Michael O. ; Bracken, Abigail J. ; Kampf, Jeff W. ; Speelman, Amy L. ; Alp, E. Ercan ; Hu, Michael Y. ; Zhao, Jiyong ; Lehnert, Nicolai ( March 2022 , Journal of the American Chemical Society)

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The Oxo-Wall Remains Intact: A Tetrahedrally Distorted Co(IV)–Oxo Complex

https://doi.org/10.1021/jacs.1c04919

Yang, Jindou ; Dong, Hai T. ; Seo, Mi Sook ; Larson, Virginia A. ; Lee, Yong-Min ; Shearer, Jason ; Lehnert, Nicolai ; Nam, Wonwoo ( October 2021 , Journal of the American Chemical Society)

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Exploring the Limits of Dative Boratrane Bonding: Iron as a Strong Lewis Base in Low-Valent Non-Heme Iron-Nitrosyl Complexes

https://doi.org/10.1021/acs.inorgchem.0c01686

Dong, Hai T. ; Chalkley, Matthew J. ; Oyala, Paul H. ; Zhao, Jiyong ; Alp, E. Ercan ; Hu, Michael Y. ; Peters, Jonas C. ; Lehnert, Nicolai ( October 2020 , Inorganic Chemistry)
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Iron and manganese oxo complexes, oxo wall and beyond

https://doi.org/10.1038/s41570-020-0197-9

Larson, Virginia A. ; Battistella, Beatrice ; Ray, Kallol ; Lehnert, Nicolai ; Nam, Wonwoo ( January 2020 , Nature Reviews Chemistry)

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